Simulated rainfall and overland-flow experiments are useful for enhancing understanding of surface hydrologic and erosion processes, quantifying runoff and erosion rates, and developing and testing predictive quantitative models. This extensive dataset consists of rainfall simulation and overland flow experimental plot data coupled with associated measures of vegetation, ground cover, and surface soil properties across point to hillslope scales. Data were collected at three woodland-encroached sagebrush (*Artemisia* spp.) rangelands in the Great Basin, USA, under undisturbed/untreated conditions and 1 yr to 9 yr following fire and/or mechanical tree-removal treatments.